{"id":206330,"date":"2025-02-13T03:22:37","date_gmt":"2025-02-13T09:22:37","guid":{"rendered":"https:\/\/lifeboat.com\/blog\/2025\/02\/electro-optic-cavities-for-in-situ-measurement-of-cavity-fields"},"modified":"2025-02-13T03:22:37","modified_gmt":"2025-02-13T09:22:37","slug":"electro-optic-cavities-for-in-situ-measurement-of-cavity-fields","status":"publish","type":"post","link":"https:\/\/lifeboat.com\/blog\/2025\/02\/electro-optic-cavities-for-in-situ-measurement-of-cavity-fields","title":{"rendered":"Electro-optic cavities for in-situ measurement of cavity fields"},"content":{"rendered":"<p><a class=\"aligncenter blog-photo\" href=\"https:\/\/lifeboat.com\/blog.images\/electro-optic-cavities-for-in-situ-measurement-of-cavity-fields.jpg\"><\/a><\/p>\n<p>Our hybrid EOC design extends these concepts by providing continuous tunability and the potential for adding active samples for investigations of intra-cavity light-matter interactions. In the \u2018empty\u2019 hybrid cavity investigated here, we observe a rich mode structure, spurring development of both a field-based model to quantify these cavity modes and their properties, as well as a complementary coupled-oscillator description to gain further understanding of the delicate interplay between the various sub-cavities, which thereafter constitute the hybrid EOC modes. Our detailed analysis of these theoretical vantage points will be highly valuable when considering the addition of an active material, after which the hybrid cavity optical response will become even more intricate. Integration of active materials into hybrid EOCs will yield novel access to light-matter interactions\u2014namely access to energy exchange on sub-Rabi-cycle timescales, and furthermore local probing and even control over tunable light-matter superposition\u2014the latter two unavailable when viewed by conventional cavity transmission techniques. Potential \u2018active materials\u2019 for these in-situ investigations of tunable light-matter interactions include conventional polar semiconductors<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 40\" title=\"Juraschek, D. M. & Narang, P. Highly confined phonon polaritons in monolayers of perovskite oxides. Nano Lett. 21, 5098&ndash;5104 (2021).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR40\" id=\"ref-link-section-d89689229e2369\">40<\/a><\/sup>\u2014oftentimes displaying very large oscillator strengths\u2014atomically-thin monolayers or heterostructures ofion-metal dichalcogenides<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 41\" title=\"Liu, F. et al. Disassembling 2D van der Waals crystals into macroscopic monolayers and reassembling into artificial lattices. Science 367903&ndash;906 (2020).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR41\" id=\"ref-link-section-d89689229e2373\">41<\/a><\/sup>, hybrid organic-inorganic 3D<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 21\" title=\"Di Virgilio, L. et al. Controlling the electro-optic response of a semiconducting perovskite coupled to a phonon-resonant cavity. Light Sci. Appl. 12,183 (2023).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR21\" id=\"ref-link-section-d89689229e2377\">21<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 42\" title=\"Frenzel, M. et al. Nonlinear terahertz control of the lead halide perovskite lattice. Sci. Adv. 9, aadg3856 (2023).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR42\" id=\"ref-link-section-d89689229e2380\">42<\/a><\/sup> and 2D lead-halide perovskites<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 43\" title=\"Chen, X. H. et al. Impact of layer thickness on the charge carrier and spin coherence lifetime in two-dimensional layered perovskite single crystals. ACS Energy Lett. 3, 2273&ndash;2279 (2018).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR43\" id=\"ref-link-section-d89689229e2384\">43<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 44\" title=\"Zhang, Z. Q. et al. Discovery of enhanced lattice dynamics in a single-layered hybrid perovskite. Sci. Adv. 9, eadg4417 (2023).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR44\" id=\"ref-link-section-d89689229e2387\">44<\/a><\/sup>, and novel, magnetically-ordered systems<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 45\" title=\"Mak, K. F., Shan, J. & Ralph, D. C. Probing and controlling magnetic states in 2D layered magnetic materials. Nat. Rev. Phys. 1646&ndash;661 (2019).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR45\" id=\"ref-link-section-d89689229e2391\">45<\/a><\/sup>.<\/p>\n<p>Implementation of EO sampling inside of THz cavities will also significantly advance further areas of contemporary research. As a prominent example, field-resolved probing inside a defined electromagnetic cavity will provide novel opportunities for measurements of electromagnetic vacuum field fluctuations<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 46\" title=\"Benea-Chelmus, I. C. et al. Electric field correlation measurements on the electromagnetic vacuum state. Nature 568202&ndash;206 (2019).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR46\" id=\"ref-link-section-d89689229e2398\">46<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 47\" title=\"Riek, C. et al. Direct sampling of electric-field vacuum fluctuations. Science 350420&ndash;423 (2015).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR47\" id=\"ref-link-section-d89689229e2401\">47<\/a><\/sup>. Most notably, a high-quality factor EOC constitutes an advantageous testing ground for measurement of quantum vacuum fluctuations, by efficiently excluding sources of external radiation. Moreover, EOCs are not limited to either macroscopic environments or the THz spectral region. Although EO sampling is routinely employed up to the mid-IR spectral region<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 9\" title=\"Sell, A., Leitenstorfer, A. & Huber, R. Phase-locked generation and field-resolved detection of widely tunable terahertz pulses with amplitudes exceeding 100 MV\/cm. Opt. Lett. 33, 2767&ndash;2769 (2008).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR9\" id=\"ref-link-section-d89689229e2405\">9<\/a><\/sup>, it has recently been extended even into the visible range<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 48\" title=\"Ridente, E. et al. Electro-optic characterization of synthesized infrared-visible light fields. Nat. Commun. 13, 1111 (2022).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR48\" id=\"ref-link-section-d89689229e2409\">48<\/a><\/sup>, allowing for future broadband measurements of intra-cavity electric fields. Similar sampling techniques have been used to sample electric fields inside of metallic antenna-based cavities<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 49\" title=\"Benea-Chelmus, I. C. et al. Electro-optic interface for ultrasensitive intracavity electric field measurements at microwave and terahertz frequencies. Optica 7498&ndash;505 (2020).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR49\" id=\"ref-link-section-d89689229e2413\">49<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 50\" title=\"Kipp, G. et al. Cavity electrodynamics of van der Waals heterostructures. arXiv https:\/\/arxiv.org\/abs\/2403.19745 (2024).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR50\" id=\"ref-link-section-d89689229e2416\">50<\/a><\/sup>, demonstrating that although on-chip photonic implementations lack the dynamic tunability, the general technique is readily implemented in other near-field contexts, including even tip-based nano-photonic applications<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 51\" title=\"M\u00fcller, M. et al. Phase-resolved detection of ultrabroadband THz pulses inside a scanning tunneling microscope junction. ACS Photonics 7, 2046&ndash;2055 (2020).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR51\" id=\"ref-link-section-d89689229e2420\">51<\/a><\/sup>. Furthermore, EOCs utilizing quartz are uniquely suited candidates for chiral THz cavity phenomena<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 52\" title=\"H\u00fcbener, H. et al. Engineering quantum materials with chiral optical cavities. Nat. Mater. 20438&ndash;442 (2021).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR52\" id=\"ref-link-section-d89689229e2425\">52<\/a><\/sup>, due to quartz\u2019s capability for straightforward and rapid measurement of vectorial electric field trajectories<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 34\" title=\"Frenzel, M. et al. Quartz as an accurate high-field low-cost THz helicity detector. Optica 11362&ndash;370 (2024).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR34\" id=\"ref-link-section-d89689229e2429\">34<\/a><\/sup>.<\/p>\n<p>In conclusion, we have established versatile and compact designs for a new class of active THz cavities, which allow for in-situ retrieval of intra-cavity electric fields. By developing a cavity-correction function formalism for these EOCs, we have demonstrated a rigorous and reliable method to extract absolute fields in a quantitative, and phase-resolved manner. Utilizing straightforward fabrication techniques, we tune the cavities\u2019 quality factors and resonance frequencies. Furthermore, we have introduced a hybrid EOC, offering continuously-tunable cavity modes across the entire THz-frequency range, within a single device. This fundamental advancement lays the groundwork for accommodating additional active materials for in-situ measurement of and control over light-matter coupling. We understand the rich hybrid mode structure, including apparent signatures of strong coupling, via cavity-field and coupled-oscillator formalisms, which will be key to deciphering signatures of light-matter coupling in more complicated devices. Therefore, this work opens new dimensions of THz cavity physics, particularly in the realms of cavity-controlled ground-and excited state material properties. This includes possibilities such as cavity-enhanced THz emission, selectively-driven Floquet states<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 53\" title=\"H\u00fcbener, H., De Giovannini, U. & Rubio, A. Phonon driven floquet matter. Nano Lett. 18, 1535&ndash;1542 (2018).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR53\" id=\"ref-link-section-d89689229e2436\">53<\/a><\/sup>, and cavity-controlled nonlinear THz driving<sup><a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 15\" title=\"Juraschek, D. M. et al. Cavity control of nonlinear phononics. Phys. Rev. Res. 3, L032046 (2021).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR15\" id=\"ref-link-section-d89689229e2440\">15<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 54\" title=\"Mornhinweg, J. et al. Tailored subcycle nonlinearities of ultrastrong light-matter coupling. Phys. Rev. Lett. 126, 177404 (2021).\" href=\"https:\/\/www.nature.com\/articles\/s41377-024-01685-x#ref-CR54\" id=\"ref-link-section-d89689229e2443\">54<\/a><\/sup>, thus paving the way for comprehensive investigations of THz cavity quantum electrodynamics.<\/p>\n","protected":false},"excerpt":{"rendered":"<p>Our hybrid EOC design extends these concepts by providing continuous tunability and the potential for adding active samples for investigations of intra-cavity light-matter interactions. In the \u2018empty\u2019 hybrid cavity investigated here, we observe a rich mode structure, spurring development of both a field-based model to quantify these cavity modes and their properties, as well as [\u2026]<\/p>\n","protected":false},"author":427,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[1523,4,1617],"tags":[],"class_list":["post-206330","post","type-post","status-publish","format-standard","hentry","category-computing","category-nanotechnology","category-quantum-physics"],"_links":{"self":[{"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/posts\/206330","targetHints":{"allow":["GET"]}}],"collection":[{"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/posts"}],"about":[{"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/users\/427"}],"replies":[{"embeddable":true,"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/comments?post=206330"}],"version-history":[{"count":0,"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/posts\/206330\/revisions"}],"wp:attachment":[{"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/media?parent=206330"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/categories?post=206330"},{"taxonomy":"post_tag","embeddable":true,"href":"https:\/\/lifeboat.com\/blog\/wp-json\/wp\/v2\/tags?post=206330"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}